Optical Hall absorption sum rule and spectral compensation in time-reversal-breaking moiré and Hofstadter systems
TLDR
This paper formulates an optical Hall absorption sum rule, linking low and high-frequency spectral contributions in time-reversal-breaking topological systems.
Key contributions
- Formulates a first-frequency-moment sum rule for antisymmetric optical conductivity.
- Shows the sum rule vanishes for zero-field moiré systems, implying spectral compensation.
- Demonstrates a universal sum rule value for Hofstadter models under uniform magnetic fields.
- Provides a rigorous framework for quantifying circular dichroism and diagnosing Landau-level mixing.
Why it matters
This work addresses a gap in understanding antisymmetric Hall absorption in topological systems. It provides a rigorous theoretical framework for interpreting experimental optical spectroscopy, crucial for advancing topological quantum states and modern materials.
Original Abstract
Optical spectroscopy provides a powerful, contact-free probe of topological quantum states, yet exact constraints on antisymmetric Hall absorption remain much less well developed than their longitudinal counterparts. Motivated by earlier Hall-conductivity sum rules, we formulate the corresponding first-frequency-moment constraint for the antisymmetric optical conductivity, whose imaginary part governs chirality-dependent absorption. We then demonstrate this sum rule in two classes of time-reversal-breaking topological systems. For a zero-field moiré continuum model hosting topological bands, the moment vanishes exactly, implying that any low-frequency anomalous Hall absorption must be compensated by higher-frequency spectral weight of the opposite sign. For a Hofstadter model under a uniform magnetic field, the same moment takes a universal value fixed by the magnetic flux density, independent of microscopic model details. By linking low- and high-frequency spectral contributions, this optical Hall absorption sum rule provides a rigorous framework for quantifying circular dichroism constraints and diagnosing Landau-level mixing. Our results show how a known Hall spectral constraint acquires new and experimentally relevant content in modern interacting topological materials.
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